期刊
CHEMISTRY-A EUROPEAN JOURNAL
卷 18, 期 31, 页码 9452-9474出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/chem.201201329
关键词
C?H activation; natural products; synthetic methods; total synthesis; transition metals
资金
- National Research Foundation of Korea (NRF) [2010-0017149, 2010-0007737]
- Ministry of Education, Science and Technology (MEST)
- National Research Foundation of Korea [2009-0063856, 2010-0007737] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)
The recent advent of transition-metal mediated C?H activation is revolutionizing the synthetic field and gradually infusing a C?H activation mind-set in both students and practitioners of organic synthesis. As a powerful testament of this emerging synthetic tool, applications of C?H activation in the context of total synthesis of complex natural products are beginning to blossom. Herein, recently completed total syntheses showcasing creative and ingenious incorporation of C?H activation as a strategic manoeuver are compared with their non-C?H activation counterparts, illuminating a new paradigm in strategic synthetic design.
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