期刊
CHEMISTRY-A EUROPEAN JOURNAL
卷 16, 期 27, 页码 8012-8019出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/chem.200903450
关键词
esters; EXAFS spectroscopy; gold; oxidation; pyridines
资金
- Deutsche Forschungsgemeinschaft (DFG) [SFB 706]
Gold complexes were prepared and investigated as catalysts for the oxidative esterification of aldehydes. Stabilisation by pyridine ligands gave good conversions and the in situ extended X-ray absorption fine structure (EXAFS) study of the reactions indicated that the reaction mixtures contained only mononuclear gold species. Thus, this is the first proof for a homogeneous gold-catalysed oxidation reaction; the presence of nanoparticles could be excluded experimentally.
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