期刊
CHEMISTRY-A EUROPEAN JOURNAL
卷 16, 期 1, 页码 276-281出版社
WILEY-BLACKWELL
DOI: 10.1002/chem.200902104
关键词
CO2 adsorption; dynamic structures; gated sorption; hysteresis; metal-organic frameworks; porous materials
资金
- Argonne National Laboratory
- U.S. Dept. of Energy [DE-FG02-08ER15967]
- Northwestern Nanoscale Science and Engineering Center
- U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]
- Midwest Universities Collaborative Access Team (MUCAT)
- Ames Laboratory [W-7405-Eng-82]
A new, twofold interpenetrated metal-organic framework (MOF) material has been synthesized that demonstrates dramatic steps in the adsorption and hysteresis in the desorption of CO2 Measurement of the structure by powder X-ray diffraction (PXRD) and pair distribution function (PDF) analysis indicates that structural changes upon CO2 sorption most likely involve the interpenetrated frameworks moving with respect to each other.
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