期刊
CHEMISTRY OF MATERIALS
卷 24, 期 13, 页码 2566-2571出版社
AMER CHEMICAL SOC
DOI: 10.1021/cm301190c
关键词
tetrabenzocoronenes; single crystal field-effect transistors
资金
- National Science Council, Taiwan, Republic of China [NSC-98-2119-M-001-007-MY3, NSC-100-2113-M-001-005-MY3]
- Academia Sinica
A series of contorted tetrabenzo[a,d,j,m]-coronenes (TBCs) substituted with four fluoro-, chloro-, or methyl groups at 2,7,12,17-positions were synthesized and characterized. Except for the one with methyl substituents, which exhibits a shifted pi-pi stacking, the rest all show cofacial pi-pi. stacking with small parallel displacements. One-dimensional growth along the stacking direction was observed in the single crystals for all derivatives. A systematic comparison of the crystal packing and the calculated electronic coupling/mobility with the measured field-effect mobility for single-crystal field-effect transistors shows a good correlation.
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