期刊
CHEMISTRY OF MATERIALS
卷 21, 期 5, 页码 934-938出版社
AMER CHEMICAL SOC
DOI: 10.1021/cm803248j
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资金
- National Science Foundation [NSF-CBET 0824361, 3M]
- Directorate For Engineering
- Div Of Chem, Bioeng, Env, & Transp Sys [0824361] Funding Source: National Science Foundation
Organic-inorganic nanocomposites consisting of electroactive conjugated polymer, poly(3-hexylthiophene) (P3HT), intimately tethered on the surface of semiconductor CdSe quantum dot (i.e., P3HT-CdSe nanocomposites) at the air/water interface formed via Langmuir isotherms were explored for the first time. The P3HT-CdSe nanocomposites displayed a high pressure plateau (similar to 10.5 mN/m) in the Langmuir isotherm, illustrating their complex packing at the air/water interface. The packing of the Langmuir-Blodgett (LB) depositions of nanocomposites was revealed by AFM measurements. Furthermore, photovoltaic devices fabricated from the LB depositions of the P3HT-CdSe nanocomposites exhibited a relatively high short circuit current, I-sc, while maintaining a thin film profile. These studies provide insights into the fundamental behaviors of semiconductor organic-inorganic nanocomposites confined at the air/water interface as well as in the active layer of an organic-based photovoltaic device.
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