期刊
CHEMISTRY LETTERS
卷 40, 期 10, 页码 1140-1142出版社
CHEMICAL SOC JAPAN
DOI: 10.1246/cl.2011.1140
关键词
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资金
- Ministry of Education, Culture, Sports, Science and Technology, Japan
- Asahi Glass Foundation
- Kansai Research Foundation
- Toyota Physical and Chemical Research Institute
- Grants-in-Aid for Scientific Research [21106001] Funding Source: KAKEN
A nickel-catalyzed cycloaddition of aromatic (O-benzyl)ketoximes with alkynes to afford 3,4-disubstituted isoquinoline derivatives has been developed. The reaction involves oxidative addition of N-O bond of O-benzylketoxime to Ni(0) and subsequent intermolecular C-H bond activation via elimination of benzyl alcohol. It was also found that ketoximes participate in the nickel-catalyzed reaction with alkynes to furnish isoquinoline N-oxide derivatives.
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