期刊
CHEMICAL SOCIETY REVIEWS
卷 42, 期 1, 页码 63-76出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c2cs35316d
关键词
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The merged inverse-electron-demand hetero-Diels-Alder (ihDA)/retro-Diels-Alder (rDA) reaction sequence can be used to rapidly synthesise highly functionalised nitrogen heteroaromatics. The reaction offers many advantages: high atom economy, high levels of regioselectivity, it rarely requires a catalyst and, in some cases, can be performed in the absence of solvent. In this tutorial review we discuss the range of commonly used dienophiles and aza-dienes for this process whilst highlighting the reactivity trends, and illustrating their applications.
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