期刊
CHEMICAL SOCIETY REVIEWS
卷 41, 期 6, 页码 2036-2051出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c1cs15278e
关键词
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资金
- U.S. Department of Energy [DE-AC02-98CH10886]
- Division of Chemical Sciences, Geosciences, & Biosciences, Office of Basic Energy Sciences under its Solar Energy Utilization initiative
- Toyota Motor Engineering & Manufacturing of North America, Inc.
In our developing world, carbon dioxide has become one of the most abundant greenhouse gases in the atmosphere. It is a stable, inert, small molecule that continues to present significant challenges toward its chemical activation as a useful carbon end product. This tutorial review describes one approach to the reduction of carbon dioxide to carbon fuels, using cobalt and nickel molecular catalysts, with particular focus on studying the thermodynamics and kinetics of CO2 binding to metal catalytic sites.
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