期刊
CHEMICAL SOCIETY REVIEWS
卷 40, 期 7, 页码 3525-3537出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c0cs00220h
关键词
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资金
- Junta de Andalucia [P09-FQM-4571]
- UGR
- Chemistry at Spin Centers [SFB 813]
This tutorial review highlights the development of radical-based bioinspired synthesis of terpenes from the initial proposal to the development of modern catalytic methods for performing such processes. The power of the radical approach is demonstrated by the straightforward syntheses of many natural products from readily available starting materials. The efficiency of these processes nicely complements the described cationic polyolefin cyclisations and even suggests that modern radical methods provide means to improve upon nature's synthetic pathways.
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