期刊
CHEMICAL SOCIETY REVIEWS
卷 38, 期 1, 页码 115-164出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/b804321n
关键词
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资金
- Division Of Chemistry
- Direct For Mathematical & Physical Scien [911558] Funding Source: National Science Foundation
A critical review of light-driven interfacial charge-transfer reactions of transition-metal compounds anchored to mesoporous, nanocrystalline TiO2 (anatase) thin films is described. The review highlights molecular insights into metal-to-ligand charge transfer (MLCT) excited states, mechanisms of interfacial charge separation, inter- and intra-molecular electron transfer, and interfacial charge-recombination processes that have been garnered through various spectroscopic and electrochemical techniques. The relevance of these processes to optimization of solar-energy-conversion efficiencies is discussed (483 references).
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