期刊
CHEMICAL PHYSICS
卷 360, 期 1-3, 页码 110-115出版社
ELSEVIER
DOI: 10.1016/j.chemphys.2009.04.019
关键词
Two-dimensional spectroscopy; Phase cycling; Nonlinear optical spectroscopy
资金
- Ministry of Education Academic Research Fund Tier I [RG 47/07]
- DSO National Laboratories
We present phase cycling schemes for two-dimensional (2D) optical spectroscopy with a pump-probe beam geometry. We detail the theoretical derivation on how the phase cycling schemes measure a pure absorptive 2D spectrum. The 'rotating frame' is inherent in such phase locked phase cycling experiments, and can increase the efficiency of the experiment by reducing the number of data points needed to be collected. 2D optical spectra are simulated for the phase cycling pump-probe experiment by solving the Liouville equation that describes the system-field interaction using a non-perturbative method. (C) 2009 Elsevier B.V. All rights reserved.
作者
我是这篇论文的作者
点击您的名字以认领此论文并将其添加到您的个人资料中。
推荐
暂无数据