期刊
CHEMICAL COMMUNICATIONS
卷 50, 期 72, 页码 10390-10393出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c4cc03946g
关键词
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资金
- U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES) [DE-FG02-13ER46972]
- NSF [CHE 1213795]
A new biomimetic heterogeneous photocatalyst ([FeFe]@ ZrPF) has been synthesized through the incorporation of homogeneous complex 1 [(i-SCH2)(2)NC(O)C5H4N]-[Fe-2(CO)(6)] into the highly robust zirconium-porphyrin based metal-organic framework (ZrPF). The immobilized biomimetic [Fe2S2] catalyst inside the MOF shows great improvement in hydrogen generation compared to the reference homogeneous catalyst complex 1.
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