期刊
CHEMICAL COMMUNICATIONS
卷 50, 期 40, 页码 5316-5318出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c3cc47542e
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资金
- University of South Florida
Self-assembly of the custom-designed octatopic porphyrin ligand of tetrakis(3,5-dicarboxybiphenyl) porphine with the in situ generated Cu-2(CO2)(4) paddlewheel moieties afforded a porous metalmetalloporphyrin framework, MMPF-9, which features a high density of Cu(II) sites confined within nanoscopic channels and demonstrates excellent performances as a heterogeneous Lewis-acid catalyst for chemical fixation of CO2 to form carbonates at room temperature under 1 atm pressure.
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