期刊
CHEMICAL COMMUNICATIONS
卷 50, 期 17, 页码 2104-2107出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c3cc49029g
关键词
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资金
- Office of Energy Efficiency and Renewable Energy
- Vehicle Technologies Program
- U.S. Department of Energy (DOE)
- Fluid Interface Reactions Structures and Transport (FIRST) Center, and Energy Frontier Research Center
- Office of Basic Energy Sciences (BES)-DOE
- laboratory directed research and development (LDRD) program at Pacific Northwest National Laboratory (PNNL)
- Joint Center for Energy Storage Research (JCESR)
- Energy Innovation Hub funded by BES-DOE
Deposition of Li is a major safety concern existing in Li-ion secondary batteries. Here we perform the first in situ high spatial resolution measurement coupled with real-time quantitative electrochemistry to characterize SEI formation on gold using a standard battery electrolyte. We demonstrate that a dendritic SEI forms prior to Li deposition and that it remains on the surface after Li electrodissolution.
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