期刊
CHEMICAL COMMUNICATIONS
卷 50, 期 5, 页码 521-523出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c3cc45025b
关键词
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资金
- European Commission [FP7-REGPOT-2008-1, 229927]
- Ministry of Education, GSRT [MIS 377252]
- EPSRC (UK), E-Futures DTC
- University of Sheffield and its Strategic Development fund
A combination of noble-metal free components, a water soluble porphyrin photosensitizer zinc meso-tetrakis(1-methylpyridinium-4-yl)porphyrin chloride [ZnTMPyP4+]Cl-4 (1) with cobaloxime complex [Co-III(dmgH)(2)(py)Cl] (2) as a catalyst, creates an efficient system for photochemical hydrogen production acting under visible light with 280 TONs. This is the first example of a water soluble porphyrin acting as a photosensitizer for cobaloxime catalysed H-2 production.
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