期刊
CHEMICAL COMMUNICATIONS
卷 50, 期 61, 页码 8412-8415出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c4cc03439b
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资金
- National Natural Science Foundation of China [21272028, 21202013]
- Innovation & Entrepreneurship Talents Introduction Plan of Jiangsu Province
- Natural Science Foundation of Zhejiang Province [R4110294]
- State Key Laboratory of Coordination Chemistry of Nanjing University
- Jiangsu Key Laboratory of Advanced Catalytic Materials Technology
- Jiangsu Province Key Laboratory of Fine Petrochemical Engineering
- Priority Academic Program Development of Jiangsu Higher Education Institutions
Copper-promoted N-cyanation of aliphatic sec-amine by CuCN is achieved via oxidative coupling. This procedure employs O-2 as a clean oxidant. Notably, sulfoximines and 1,1,3,3-tetramethylguanidine also worked well in this procedure. Thus, it represents a key progress in the C-N bond formation reaction as well as in the cyanation reaction.
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