期刊
CHEMICAL COMMUNICATIONS
卷 50, 期 40, 页码 5294-5297出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c3cc47873d
关键词
-
资金
- Ministry of Science Technology [2013CB836900]
- National Natural Science Foundation of China [21290180, 21172235, 21222202]
An efficient approach toward the synthesis of the 6,6,5,7-tetracyclic core of the daphnilongeranin B, a Daphniphyllum alkaloid, is reported. The bridged 6,6-bicyclic system was constructed using a gold(I) catalysed Conia-ene reaction, while the 5-and 7-membered rings were assembled by two diastereoselective Michael addition reactions, respectively.
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