期刊
CHEMICAL COMMUNICATIONS
卷 50, 期 54, 页码 7191-7194出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c4cc02852j
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Hydrolytic oxidation of organosilanes based on an iron catalyst is described for the first time. The novel iron complex, [Fe(C6H5N2O)-(CO)(MeCN)(3)][PF6], exhibits excellent mediating power in the catalytic hydrolysis of organosilanes to produce dihydrogen and organosilanols with turnover numbers approaching 10(4) and turnover frequencies in excess of 10(2) min(-1) under ambient conditions.
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