期刊
CHEMICAL COMMUNICATIONS
卷 50, 期 31, 页码 4085-4088出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c4cc00621f
关键词
-
资金
- National Nature Science Foundation of China [2127222, 91213303, 21172205, J1030412]
Oxidative coupling of methylamines with an aminyl radical to construct amides was developed in the presence of an I-2/TBHP catalyst under acidic conditions via the two cleavages of the sp(3) C-N bond of aryl-methylamines and the sp(2) C-N bond of N-substituted formamides respectively. This transition-metal-free protocol provides a novel synthetic tool for the construction of N-substituted amides and a series of arylamides can be easily obtained with good yields.
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