期刊
CHEMICAL COMMUNICATIONS
卷 50, 期 14, 页码 1722-1724出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c3cc47060a
关键词
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资金
- NSF [1255519]
- Direct For Mathematical & Physical Scien
- Division Of Chemistry [1255519] Funding Source: National Science Foundation
Au144-xCux(SR)(60) alloy nanomolecules were synthesized and characterized by using ESI-MS to atomic precision. A maximum of 23 copper atoms replace the gold atoms. When the number of copper atoms is higher than eight, a surface plasmon-like peak appears at similar to 520 nm. Based on the fundamental elemental properties of Au and Cu, we predict a mixed atomic ordering and incorporation of Cu atoms into the Au-12 and Au-42 shells of the proposed icosahedral structure model of the 144-atom nanomolecule.
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