4.7 Article

An organocatalytic asymmetric sequential allylic alkylation-cyclization of Morita-Baylis-Hillman carbonates and 3-hydroxyoxindoles

期刊

CHEMICAL COMMUNICATIONS
卷 49, 期 82, 页码 9422-9424

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ROYAL SOC CHEMISTRY
DOI: 10.1039/c3cc45139a

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  1. National Natural Science Foundation of China [21272230]
  2. Western Light Talent Culture Project

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The first organocatalytic asymmetric sequential allylic alkylationcyclization of Morita-Baylis-Hillman carbonates and 3-hydroxyoxindoles has been developed to afford spirooxindoles bearing alpha-methylene-gamma-butyrolactone motifs in 25-85% yield, 60-94% ee and up to > 20:1 diastereoselectivity.

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