期刊
CHEMICAL COMMUNICATIONS
卷 49, 期 78, 页码 8824-8826出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c3cc44399j
关键词
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资金
- Institute for Advanced Studies in Basic Sciences
- National Elite Foundation
Nanolayered Mn oxide/poly(4-vinylpyridine) as a model for Mn cluster in photosystem II was synthesized and characterized using scanning electron microscopy (SEM), transmission electron microscopy (TEM), dynamic light scattering (DLS), Fourier transform infrared spectroscopy (FTIR) and UV-Visible spectroscopy (UV-Vis). The compound is a very efficient water oxidizing catalyst, and sizable oxygen evolution was detected at 50 mV overpotential at near neutral pH. The number is as low as the overpotential is used by nature in photosystem II of cyanobacteria, algae and green plants for similar reactions.
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