期刊
CHEMICAL COMMUNICATIONS
卷 48, 期 43, 页码 5280-5282出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c2cc31523h
关键词
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Hypervalent N-triflylimino-lambda(3)-bromane undergoes direct and regioselective alpha-C-H amination of ethers at room temperature under transition metal-free conditions. Kinetic results, substituent and deuterium isotope effects suggest an asynchronous concerted organonitrenoid transition state with some hydride transfer character, analogous to that for alkane C-H insertions.
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