期刊
CHEMICAL COMMUNICATIONS
卷 48, 期 87, 页码 10775-10777出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c2cc34973f
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资金
- EPSRC
- National Nature Science Foundation of China [21071048]
- Chang Jiang Scholar Candidates Programme for Provincial Universities in Heilongjiang [2012CJHB003]
- Science Foundation of Harbin City of China [2011RFXXG001]
- Programme for Innovative Research Team in Heilongjiang University [Hdtd2010-02]
The surface modification with a proper amount of phosphate accelerates the dynamic decay of photogenerated electrons in the nanocrystalline anatase TiO2 film in the presence of O-2, consequently prolonging greatly the lifetime of photogenerated holes so as to improve the charge separation of TiO2 and then its photocatalytic activity for degrading gas-phase acetaldehyde and liquid-phase phenol mainly based on the transient absorption spectra and the measurements of electrochemical O-2 reduction and the produced hydroxyl radical amount. The acceleration effects are attributed to the increased amount of adsorbed O-2 by means of the curves of O-2 temperature-programmed desorption.
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