期刊
CHEMICAL COMMUNICATIONS
卷 48, 期 2, 页码 272-274出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c1cc16024a
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The light-assisted co-generation of carbon monoxide and hydrogen from carbon dioxide and water is reported. The combination of a homogeneous CO-evolving electrocatalyst and a heterogeneous H-2-evolving photoelectrode surface provides for tunability of the H-2/CO ratio. A total Faradaic efficiency of 102 +/- 5% and a H-2/CO ratio of 2 : 1 were achieved at a low homogeneous catalyst concentration (0.5 mM) in acetonitrile/water mixtures.
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