期刊
CHEMICAL COMMUNICATIONS
卷 47, 期 33, 页码 9268-9274出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c1cc12390d
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The efficient storage of solar energy in chemical fuels, such as hydrogen, is essential for the large-scale utilisation of solar energy systems. Recent advances in the photocatalytic production of H-2 are highlighted. Two general approaches for the photocatalytic hydrogen generation by homogeneous catalysts are considered: HX (X = Cl, Br) splitting involving both proton reduction and halide oxidation via an inner-sphere mechanism with a single-component catalyst; and sensitized H-2 production, employing sacrificial electron donors to regenerate the active catalyst. Future directions and challenges in photocatalytic H-2 generation are enumerated.
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