期刊
CHEMICAL COMMUNICATIONS
卷 47, 期 29, 页码 8406-8408出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c1cc12200b
关键词
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资金
- Solar Energy Initiative of the Chinese Academy of Sciences [KGCXZ-YW-389]
- National Natural Science Foundation of China [20732007, 21090343, 50973125]
- Ministry of Science and Technology of China [G2007CB808004, 2009CB22008]
- Bureau for Basic Research of the Chinese Academy of Sciences
A novel molecular triad [FeFe]-H(2)ase 1, and its model complexes 2 and 3 have been successfully constructed. The multistep PET and long-lived Fe(I)Fe(0) species were found to be responsible for the better performance of triad 1 than that of 2 with 3 for light-driven H-2 evolution.
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