期刊
CHEMICAL COMMUNICATIONS
卷 47, 期 5, 页码 1515-1517出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c0cc04447d
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资金
- MEXT, Japan
Efficient catalytic asymmetric synthesis of 1,1-disubstituted tetrahydro-beta-carbolines has been achieved via asymmetric alkylation of 1-cyanotetrahydro-beta-carbolines using a binaphthyl-modified N-spiro-type chiral phase-transfer catalyst. This is a valuable example of hitherto difficult highly enantioselective alkylations at alpha-carbon of the cyano group under phase-transfer conditions.
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