4.7 Article

Synthesis and structure of [{N(CH2CH2NSiMe3)(3)}URe(eta(5)-C5H5)(2)]: a heterobimetallic complex with an unsupported uranium-rhenium bond

期刊

CHEMICAL COMMUNICATIONS
卷 -, 期 20, 页码 2851-2853

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ROYAL SOC CHEMISTRY
DOI: 10.1039/b906554g

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资金

  1. EPSRC [EP/G051763/1, EP/F030517/1] Funding Source: UKRI
  2. Engineering and Physical Sciences Research Council [EP/G051763/1, EP/F030517/1] Funding Source: researchfish

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The first structurally authenticated molecular uranium-transition metal bond is reported; DFT studies show sigma- and pi-components in the U-Re bond and this is the first time that the latter component has been reported in an unsupported f-element-transition metal bond.

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