期刊
CHEMICAL COMMUNICATIONS
卷 -, 期 46, 页码 7206-7208出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/b916640h
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资金
- Swedish Research Council
- Goran Gustafssons Foundation
- Carl Trygger Foundation
- Uppsala University through the U<SUP>3</SUP>MEC molecular electronics priority initiative
C,C-Diacetylenic phosphaalkenes have been obtained from a 1-chloro-3-ethynyl-1,2-allene which becomes accessible from a silica-promoted rearrangement of a 3-chloropenta-1,4-diyne; oxidative acetylene homo-coupling of the phosphadiethynyl-ethene is described for the first time and affords a dimeric, cross-conjugated product which features a largely decreased HOMO-LUMO gap compared to all-carbon-based reference compounds.
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