期刊
CHEMICAL COMMUNICATIONS
卷 -, 期 40, 页码 4986-4988出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/b806075d
关键词
-
资金
- Seaborg Institute
- Division of Chemical Sciences
- Office of Basic Energy Sciences
- US Department of Energy
The bis(imido) uranium(VI)-C(5)H(5) and -C(5)Me(5) complexes (C(5)H(5))(2)U(N(t)Bu)(2), (C(5)Me(5))(2)U(N(t)Bu)(2), (C(5)H(5))U(N(t)Bu)(2)(I)-(dmpe), and (C(5)H(5))(2)U(N(t)Bu)(2)(dmpe) can be synthesized from reactions between U(N(t)Bu)(2)(I)(2)(L)(x) (L = THF, x = 2; L = dmpe, x = 1) and Na(C(5)R(5)) (R = H, Me); these complexes represent the first structurally characterized C(5)H(5)-compounds of uranium(VI) and they further highlight the differences between UO(2)(2+) and the bis(imido) fragment.
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