期刊
CHEMICAL COMMUNICATIONS
卷 -, 期 47, 页码 6354-6356出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/b815845b
关键词
-
资金
- Japan Society of the Promotion of Science (JSPS)
A mild and efficient process for the direct-type catalytic allylation of sulfonylimidates has been developed; this reaction represents the first example of Bronsted base-catalysed, in situ generation and use of alpha-alkyl enolates in substitution reactions; the success of this methodology stems from the tunable alpha-proton acidity and nucleophilicity of sulfonylimidates, which could be harnessed in the realization of a broader range of catalytic direct-type reactions using ester equivalents as nucleophiles.
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