期刊
CHEMCATCHEM
卷 6, 期 1, 页码 91-95出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/cctc.201300763
关键词
hydrogenolysis; lignin; nickel; nanoparticles; sustainable chemistry
资金
- Deutsche Forschungsgemeinschaft [SFB 840]
- HEC Pakistan
- DAAD
SiC materials with tailored porosity and integrated Ni NPs (Ni@SiC) were synthesized via microphase separation of polycarbosilane-block-polyethylene followed by its pyrolysis. Changing the length of organic block allowed the synthesis of micro, meso and hierarchical Ni@SiC materials which were characterized by PXRD, TEM, TGA, and nitrogen physisorption. Selective hydrogenolysis of aryl ethers mimicking the most abundant linkages of lignin was achieved in water avoiding the possible hydrogenation of aromatic rings.
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