期刊
CHEMCATCHEM
卷 5, 期 7, 页码 1877-1883出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/cctc.201200957
关键词
aryl boronic acids; CH activation; indole; metal-organic frameworks; Pd nanoparticles
资金
- 973 Program [2011CB932504, 2013CB933203]
- Natural Science Foundation of China [21003128, 21273238, 21221001]
- Fujian Key Laboratory of Nanomaterials [2006L2005]
- CAS
Highly dispersed Pd nanoparticles encapsulated in the mesoporous metal-organic framework MIL-101 demonstrated high activity and selectivity for the direct C2 arylation of various indoles with aryl boronic acids using O2 or 2,2,6,6-tetramethylpiperidine N-oxyradical as an external oxidant in acidic media under mild conditions. The green catalyst is easily recoverable and can be reused six times without leaching and loss of activity.
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