期刊
CATALYSIS TODAY
卷 228, 期 -, 页码 5-14出版社
ELSEVIER
DOI: 10.1016/j.cattod.2013.12.024
关键词
Oxidative coupling of methane; OCM; MnxOy-Na2WO4/SiO2; Support material variation; Silica; TiO2-rutile
资金
- Deutsche Forschungsgemeinschaft (DFG)
MnxOy,-Na2WO4/SiO2 is an active catalyst for the oxidative coupling of methane, with a remarkable stability and a suitable performance for an industrial application. MnxOy,-Na2WO4 was supported on different support materials and the catalytic activity was investigated with a parallel reactor system, allowing a direct comparison of all results. Considering the C-2 yield and the potential practical application, SiO2 is indeed the best support material for this catalyst. However, the comparison in an X-S plot with a reference MnxOy,-Na2WO4/SiO2 catalyst indicates that SiC, Fe2O3-based oxides and TiO2-rutile are also promising support materials. (C) 2014 Elsevier B.V. All rights reserved.
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