期刊
CATALYSIS LETTERS
卷 142, 期 11, 页码 1382-1387出版社
SPRINGER
DOI: 10.1007/s10562-012-0908-z
关键词
Fischer-Tropsch synthesis; Cobalt on alumina catalyst; Product distribution; Fixed-bed and slurry-bed reactors; Catalyst deactivation
资金
- NPRP from the Qatar National Research Fund [28-6-7-32, 08-173-2-050]
The effect of CO conversion (35-91 %) on hydrocarbon product distribution (CH4, C-5(+) and olefin selectivities) and CO2 selectivity was studied in a fixed bed reactor on 15 % Co/Al2O3 catalyst at conditions of industrial relevance. Selectivity to CH4 decreased, whereas those of C-5(+) and CO2 increased with increasing CO conversion (and consequently, partial pressure of water produced during the Fischer-Tropsch synthesis). 1-Olefin content of C-2-C-5 olefins decreased and 2-olefin content of C-4 hydrocarbon increased with increasing CO conversion.
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