期刊
CATALYSIS COMMUNICATIONS
卷 28, 期 -, 页码 82-85出版社
ELSEVIER SCIENCE BV
DOI: 10.1016/j.catcom.2012.08.002
关键词
BaZrO3; Photocatalytic activity; Hydrogen generation; Water splitting
资金
- Department of Science and Technology (DST), India [SR/S1/IC-25/2009]
- Department of Atomic Energy, BRNS [2010/37P/11/BRNS]
Ta doped BaZrO3 photocatalyst with a cubic perovskite structure was synthesized using precipitation from homogenous solution method. After calcination, the obtained BaZr1-xTaxO3 (x = 0, 0.01, 0.02, 0.03. 0.04 and 0.05) samples were characterized by powder X-ray diffraction, UV-vis diffuse reflectance spectroscopy, surface area analyses and photocatalytic activity. As-prepared BaZr1-xTaxO3 samples show efficient hydrogen generation by water splitting without addition of any co-catalyst under UV-vis light irradiation. The highest hydrogen production rate (180 mu mol/h) was achieved by BaZr0.96Ta0.04O3 which could be attributed to extended absorption in visible region and surface area. (C) 2012 Elsevier B.V. All rights reserved.
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