期刊
CATALYSIS COMMUNICATIONS
卷 17, 期 -, 页码 184-188出版社
ELSEVIER
DOI: 10.1016/j.catcom.2011.11.003
关键词
Heteropoly acid; Phosphotungstic acid; Fe-bentonite; Photo-Fenton; Methyl orange
资金
- open foundation from Key Laboratory for New Processing Technology of Nonferrous Metals and Materials of the China's Ministry of Education [GXKFJ09-13]
- Guangxi Science Foundation [2011GXNSFB018017]
- China Postdoctoral Science Foundation [20110490097]
- Laboratory Construction and Experimental Teaching Reform of Guangxi University [20110305]
H3PW12O40 supported Fe-bentonite (HPW-Fe-Bent) was prepared by an impregnation method. Catalyst characterization showed H3PW12O40 and iron species were successfully immobilized on HPW-Fe-Bent. Photo-Fenton degradation of methyl orange (MO) by HPW-Fe-Bent as heterogeneous catalyst was studied. The impacts of various operating parameters on degradation ratio were analyzed. The results showed HPW-Fe-Bent used as heterogeneous catalyst in photo-Fenton process had a wide applicable range of pH and temperature. Moreover, HPW-Fe-Bent had a long-term stability for use, and retained almost all of its catalytic stability and activity after five recycling times. The possible mechanisms involving in photo-Fenton process were presented in paper. (C) 2011 Elsevier BM. All rights reserved.
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