期刊
BULLETIN OF THE CHEMICAL SOCIETY OF JAPAN
卷 77, 期 1, 页码 95-99出版社
CHEMICAL SOC JAPAN
DOI: 10.1246/bcsj.77.95
关键词
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The excited high-spin quartet (S = 3/2) state of the intramolecular triplet-radical pair between the excited triplet state of pyrene and a dangling verdazyl radical was reported. A novel verdazyl radical with the pyrene moiety was designed and synthesized. The time-resolved ESR spectrum and a DFT calculation show the photo-induced ferromagnetic spin alignment between the excited triplet state of the pyrene moiety and the dangling verdazyl radical. This is the first observation of the high-spin (S > 1) excited state of the pi-conjugated pyrene-radical pair.
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