期刊
CARBON
卷 55, 期 -, 页码 116-125出版社
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.carbon.2012.12.017
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A simple strategy for the preparation of composites with high dielectric constant and thermal conductivity was developed through a typical interface design. Graphite nanoplatelets (GNPs) with a thickness of 20-50 nm are fabricated and homogeneously dispersed in the epoxy matrix. A high dielectric constant of more than 230 and a high thermal conductivity of 0.54 W/mK (a 157% increase over that of pure epoxy) could be obtained for the composites with a lower filler content of 1.892 vol.%. The dielectric constant still remains at more than 100 even in the frequency range of 10(5)-10(6) Hz. When loaded at 2.703 vol.%, GNP/epoxy composites have a dielectric constant higher than 140 in the frequency range of 10(2)-10(4) Hz and a high thermal conductivity of 0.72 W/mK, which is a 240% increase over that of pure epoxy. The high dielectric constant and low loss tangent are observed in the composite with the GNPs content of 0.949 vol.% around 10(5)-10(6) Hz. It is believed that high aspect ratio of GNPs and oxygen functional groups on their basal planes are critical issues of the constitution of a special interface region between the GNPs and epoxy matrix and the high performance of the composites. (C) 2012 Elsevier Ltd. All rights reserved.
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