期刊
CARBON
卷 64, 期 -, 页码 141-149出版社
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.carbon.2013.07.045
关键词
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资金
- National Natural Science Foundation of China [51202004]
- Nature Science Foundation of Anhui Province [KJ2013A051]
- Foundation of Key Laboratory of Colloid and Interface Chemistry (Shangdong University), Ministry of Education [201201]
We developed a direct carbonization strategy to efficiently fabricate mesoporous N-containing carbon nanosheets (N-CNSs) by using polyaniline nanosheets as a carbon precursor. Physicochemical characterizations revealed that the as-synthesized N-CNSs with 5.9 wt.% N species possessed a well-developed mesoporous architecture with large specific surface area of 352 m(2) g(-1), high mesoporous volume of 0.32 cm(3) g(-1), and average pore size of similar to 5.2 nm. When further utilized as an electrode for electrochemical capacitors, the mesoporous N-CNSs delivered a large specific capacitance of 239 F g(-1) at 0.5 A g(-1), and even 197 F g at a high current load of 8 A g, indicating its good rate behavior. Furthermore, the capacitance degradation of e, similar to 4% over continuous 5000 charge-discharge cycles at 6 A g(-1) further verified its good electrochemical stability at high rates for long-term electrochemical capacitors application. (C) 2013 Elsevier Ltd. All rights reserved.
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