期刊
CARBON
卷 50, 期 12, 页码 4379-4387出版社
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.carbon.2012.05.014
关键词
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资金
- National Science Foundation [CMMI-0900509]
- Department of Energy [DE-EE-0003208]
- University of Wisconsin System
- UWM Research Foundation
- Innovation Program of the State Key Laboratory of Clean Energy Utilization [ZJUCEU2011009]
- Div Of Civil, Mechanical, & Manufact Inn
- Directorate For Engineering [0900509] Funding Source: National Science Foundation
We report on a one-step binder-free fabrication method for electrochemical double layer (EDL) capacitor electrodes consisting of vertically-oriented graphene uniformly grown on a metallic current collector. The double-layer capacitive behavior of the resulting electrode is studied in both aqueous and organic electrolytes. Compared with conventional graphene-based EDL capacitor electrode fabrication methods, this method offers the following advantages: (a) no need to use a binder, (b) open channels for better ion access, and (c) exposed edge planes for improved material wettability. These unique features lead to excellent capacitive behavior in organic electrolytes, including a specific capacitance slightly higher than that in aqueous electrolytes at the same potential scan rate and a high knee frequency (similar to 3174 Hz in the current work). (C) 2012 Elsevier Ltd. All rights reserved.
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