4.7 Article

A novel {Fe-I-Fe-II-Fe-II-Fe-I} iron thiolate carbonyl assembly which electrocatalyses hydrogen evolution

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CHEMICAL COMMUNICATIONS
卷 -, 期 1, 页码 133-135

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ROYAL SOC CHEMISTRY
DOI: 10.1039/b411559g

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A novel tetra-iron thiolate carbonyl assembly is described in which two dithiolate tetracarbonyl di-iron centres with a 'butterfly' configuration of the {2Fe3S}-cores are fused by two bridging thiolates which form a central planar 2Fe2S unit and comprise the first example of a chain of four metal-metal bonded iron atoms supported by a bridging sulfur framework; the assembly electrocatalyses hydrogen evolution.

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