期刊
CHEMISTRY-A EUROPEAN JOURNAL
卷 11, 期 1, 页码 112-119出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/chem.200400540
关键词
cyclic voltammetry; flavins; redox catalysis; redox chemistry
Eight different flavin derivatives have been synthesized and the electronic effects of substituents in various positions on the flavin redox chemistry were investigated. The redox potentials of the flavins, determined by cyclic voltammetry, correlated with their efficiency as catalysts in the H2O2 oxidation of methyl p-tolyl sulfide. Introduction of electron-withdrawing groups increased the stability of the reduced catalyst precursor.
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