4.7 Article

Non-Gaussian nature of glassy dynamics by cage to cage motion

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PHYSICAL REVIEW E
卷 75, 期 1, 页码 -

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AMER PHYSICAL SOC
DOI: 10.1103/PhysRevE.75.011504

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A model based on a single Brownian particle moving in a periodic effective field is used to understand the non-Gaussian dynamics in glassy systems of cage escape and subsequent recaging, often thought to be caused by a heterogeneous glass structure. The results are compared to molecular-dynamics simulations of systems with varying complexity: quasi-two-dimensional colloidlike particles, atactic polystyrene, and a dendritic glass. The model nicely describes generic features of all three topologically different systems, in particular around the maximum of the non-Gaussian parameter. This maximum is a measure for the average distance between cages.

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