期刊
ACS APPLIED MATERIALS & INTERFACES
卷 7, 期 21, 页码 11322-11329出版社
AMER CHEMICAL SOC
DOI: 10.1021/acsami.5b01706
关键词
Hemin; HKUST-1; catalysis; chemiluminescence; H2O2; glucose
资金
- National Natural Science Foundation of China [21375020, J1103303]
- Specialized Research Fund for the Doctoral Program of Higher Education of China [20133514110001]
- Program for Changjiang Scholars and Innovative Research Team in University [IRT1116]
Novel metal-organic frameworks (MOFs) based solid catalysts have been synthesized by encapsulating Hemin into the HKUST-1 MOF materials. These have been first applied in the chemiluminescence field with outstanding performance. The functionalized MOFs not only maintain an excellent catalytic activity inheriting from Hemin but also can be cyclically utilized as solid mimic peroxidases in the neutral condition. The synthesized Hemin@HKUST-1 composites have been used to develop practical sensors for H2O2 and glucose with wide response ranges and low detection limits. It was envisioned that catalyst-functionalized MOFs for chemiluminescence sensing would have promising applications in green, selective, and sensitive detection of target analytes in the future.
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