期刊
ACS APPLIED MATERIALS & INTERFACES
卷 7, 期 18, 页码 9497-9506出版社
AMER CHEMICAL SOC
DOI: 10.1021/acsami.5b00636
关键词
selective catalytic reduction; nitrogen oxides; diesel engine exhaust; thermal stability; Ce-Zr mixed oxide
资金
- National Natural Science Foundation of China [51221892]
- Ministry of Science and Technology China [2013AA065301]
A novel Mo-promoted Ce-Zr mixed oxide catalyst prepared by a homogeneous precipitation method was used for the selective catalytic reduction (SCR) of NOx with NH3. The optimal catalyst showed high NH3-SCR activity, SO2/H2O durability, and thermal stability under test conditions. The addition of Mo inhibited growth of the CeO2 particle size, improved the redox ability, and increased the amount of surface acidity, especially the Lewis acidity, all of which were favorable for the excellent NH3-SCR performance. It is believed that the catalyst is promising for the removal of NOx from diesel engine exhaust.
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