期刊
RSC ADVANCES
卷 6, 期 74, 页码 69728-69732出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c6ra15808k
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资金
- Russian Science Foundation [14-13-00445]
- FASO Russia project [0333-2014-0001]
- RSF [14-23-00146]
- Russian Science Foundation [14-23-00146] Funding Source: Russian Science Foundation
- NATIONAL INSTITUTE OF BIOMEDICAL IMAGING AND BIOENGINEERING [F32EB021840, R21EB018014, T32EB001628, R21EB020323] Funding Source: NIH RePORTER
Here, we report the production of C-13-hyperpolarized ethyl acetate via heterogeneously catalyzed pairwise addition of parahydrogen to vinyl acetate over TiO2-supported rhodium nanoparticles, followed by magnetic field cycling. Importantly, the hyperpolarization is demonstrated even at the natural abundance of C-13 isotope (ca. 1.1%) along with the easiest separation of the catalyst from the hyperpolarized liquid.
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