期刊
ORGANIC & BIOMOLECULAR CHEMISTRY
卷 16, 期 46, 页码 8884-8898出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c8ob02348d
关键词
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资金
- Ministry of Science and Technology of the People's Republic of China [2016YFA0602900]
- NSFC [21672071, 21871096]
- Natural Science Foundation of Guangdong Province [2016A030310433, 2018B030308007, 2018A030310359]
- Guangdong Province Science Foundation [2017B090903003]
- Science and Technology Program of Guangzhou [201707010316]
- China Postdoctoral Science Foundation [2018M633042]
Enynals and enynones have emerged as focal substrates in organic synthesis in view of their structure diversity, high reactivity and intermediate variety. Transition metal- or Lewis acid-promoted protocols starting from enynals/enynones could provide efficient and direct access to functionalized homo- or heterocyclic compounds. In consideration of the different electronic properties of substituents on the alkyne group of enynals/enynones, they are classified into two kinds in this review, namely donorenynals/enynones with non-electron-withdrawing substituents and acceptor-enynals/enynones with electron-withdrawing moieties. Herein we mainly introduced three kinds of transformations based on benzo-fused donor- and acceptor-enynals/enynones, including their reactions with alkenes, alkynes, and H2O, respectively.
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