期刊
ACS APPLIED MATERIALS & INTERFACES
卷 7, 期 32, 页码 17811-17818出版社
AMER CHEMICAL SOC
DOI: 10.1021/acsami.5b04118
关键词
ZnO/ZnFe2O4; double-shell; heterostructure; gas sensor; acetone
资金
- National Nature Science Foundation of China [61374218, 61134010, 61327804]
- Program for Chang Jiang Scholars and Innovative Research Team in University [IRT13018]
- National High-Tech Research and Development Program of China (863 Program) [2013AA030902, 2014AA06A505]
- Jilin University [2015094]
In this study, double-shell composites consisting of inner ZnO hollow microspheres (ZHS) surrounded by outer ZnFe2O4 nanosheets were successfully synthesized. The growth of the ultrathin ZnFe2O4 nanosheets (-10 nm) on the ZHS outer surface was carried out at room temperature via solution reactions in order to generate a double-shell configuration that could provide a large surface area. As a proof-of-concept demonstration of the design, a comparative sensing investigation between the sensors based on the asobtained ZnO/ZnFe2O4 composites and its two individual components (ZnO hollow spheres and ZnFe2O4 nanosheets) was performed. As expected, the response of the ZnFe2O4-decorated ZnO composites to 100 ppm acetone was about 3 times higher than that of initial ZnO microspheres. Moreover, a dramatic reduction of response/recover time has been achieved at different operating temperature. Such favorable sensing performances endow these ZnO/ZnFe2O4 heterostructures with a potential application in gas sensing.
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